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页岩气网络设计与运行之间的相互作用，包括CO2sub>固存

Sharifzadeh Mahdi, Xingzhi Wang, Nilay Shah

《工程（英文）》 2017年第3卷第2期页码 244-256 doi: 10.1016/J.ENG.2017.02.007

摘要：但是，由于页岩气储层的渗透率极低，因此可能需要按顺序进行特殊程序，例如水平钻井，水力压裂，定期关井和注入二氧化碳（CO 2 sub>）以提高天然气产量，最大程度地提高经济效益，并确保安全和无害环境的运营接下来，我们对重要设计和操作决策进行敏感性分析，例如井长，井眼布置，裂缝数量，裂缝距离，CO 2 sub>注入速率和闭井调度，以获取增产效果。对页岩气网络复杂行为的深入见解。结果表明，页岩气产量最高的情况不一定是最有利可图的设计。钻探，压裂和CO 2 sub>注入对这项技术的经济可行性具有重大影响。尤其是，由于成本高昂，除非使用CO 2 sub>减税或补贴，否则使用CO 2 sub>的增强气体回收（EGR）似乎不具有商业竞争力。隔离。研究还发现，设计和运营决策之间的相互作用非常重要，这些决策应同时进行优化。

关键词：页岩气，水力压裂，调度，完井，CO 2 sub>隔离，同时优化

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低渗油藏裸眼水平井压裂技术及应用

潘毓兵

《中国工程科学》 2012年第14卷第4期页码 70-73

摘要：

针对大庆外围朝长地区未动用储量属于低渗透扶余油层，采用常规直井开发，单井产能低、开发效益差，为进一步提高低渗透扶余油层开发效果，通过水平井近平衡钻井、裸眼完井，减少了钻井及固井对储层污染，采用打孔管结合油膨胀封隔器工艺进行压裂改造，探索低产低渗透储层有效的开发途径。试油及投产效果表明，低渗透油藏采用近平衡钻井、裸眼完井能有效地保护储层，实施裸眼水平井储层压裂改造能够提高单井日产油，对进一步改善低渗透油藏开发效果有重要意义。

关键词：低渗透水平井裸眼完井压裂

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固体氧化物电解池共电解H2sub>O/CO2sub>研究进展

范慧,宋世栋,韩敏芳

《中国工程科学》 2013年第15卷第2期页码 107-112

摘要：本文介绍了固体氧化物电解池的结构特点及其用于H2O/CO2的共电解制备H2和CO的工作原理，综述了固体氧化物电解池的组成形式，以及单片电解池和电解池堆用于H2O/CO2共电解反应的国内外研究进展，并阐述了提高固体氧化物电解池共电解效率所亟需解决的问题

关键词：固体氧化物电解池 H2sub>O/CO2sub>共电解合成气电解效率水电解

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山西沁水盆地柿庄北区块3#煤层注入埋藏CO2sub>提高煤层气采收率试验和评价

叶建平,张兵,Sam Wong

《中国工程科学》 2012年第14卷第2期页码 38-44

摘要：

对沁水盆地南部柿庄北区块进行了深煤层注入地质和工程评价，认为柿庄北区块适合进行深煤层注入CO2开采煤层气技术的应用；通过SX-001井的微型先导性试验，对SX-001井的注入前后产气量与产水量、气体成分变化和井底压力变化规律进行了总结。通过现场试验，注入CO2后SX-001井的产气量是注入前的2.45倍；在小于煤岩破裂压力的条件下，每天注入20 t的CO2能够实现顺利注入，并且压力上升速度较慢；注入CO2后，煤岩发生膨胀，局部煤层的渗透率降低，排采一段时间后恢复；在目的煤层中注入的CO2的影响范围内，烃类气体总的置换效率达到14.18 cm3/g。该试验成果证明柿庄北区块通过注入CO2开采煤层气实现了CO2的埋藏，提高了煤层气井的采收率。

关键词：山西沁水盆地注入CO2sub> 煤层气采收率

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山西沁水煤层气压裂施工的横向效应

李梦溪,张聪

《中国工程科学》 2012年第14卷第4期页码 16-19

摘要：

介绍了在山西沁水盆地煤层气压裂时监测到的压裂施工的横向效应，监测使用微地震方法。发现沿人工裂缝法向方向的邻井在施工时出现气量减少、枯竭、出水等反应，沿人工裂缝走向方向的邻井反应滞后。这一发现使笔者注意到煤层气压裂施工的横向挤压作用可能即时影响邻井产量，压裂设计时应该注意到这一反应的不良影响。

关键词：煤层气裂缝水力压裂

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烯烃生产新趋势

Ismaël Amghizar,Laurien A. Vandewalle,Kevin M. Van Geem,Guy B. Marin

《工程（英文）》 2017年第3卷第2期页码 171-178 doi: 10.1016/J.ENG.2017.02.006

摘要：部分上述工艺主要得益于页岩气和闲置天然气中大量廉价的丙烷乙烷和甲烷。

关键词：烯烃生产蒸汽裂解甲烷转化页岩气碳排放

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CO2sub> methanation and co-methanation of CO and CO2sub> over Mn-promoted Ni/Al2sub>O3sub> catalysts

Kechao Zhao,Zhenhua Li,Li Bian

《化学科学与工程前沿（英文）》 2016年第10卷第2期页码 273-280 doi: 10.1007/s11705-016-1563-5

摘要： A series of Mn-promoted 15 wt-% Ni/Al O catalysts were prepared by an incipient wetness impregnation method. The effect of the Mn content on the activity of the Ni/Al O catalysts for CO methanation and the co-methanation of CO and CO in a fixed-bed reactor was investigated. The catalysts were characterized by N physisorption, hydrogen temperature-programmed reduction and desorption, carbon dioxide temperature-programmed desorption, X-ray diffraction and high-resolution transmission electron microscopy. The presence of Mn increased the number of CO adsorption sites and inhibited Ni particle agglomeration due to improved Ni dispersion and weakened interactions between the nickel species and the support. The Mn-promoted 15 wt-% Ni/Al O catalysts had improved CO methanation activity especially at low temperatures (250 to 400 °C). The Mn content was varied from 0.86% to 2.54% and the best CO conversion was achieved with the 1.71Mn-Ni/Al O catalyst. The co-methanation tests on the 1.71Mn-Ni/Al O catalyst indicated that adding Mn markedly enhanced the CO methanation activity especially at low temperatures but it had little influence on the CO methanation performance. CO methanation was more sensitive to the reaction temperature and the space velocity than the CO methanation in the co-methanation process.

关键词： Mn promotion nickel catalysts CO₂ methanation co-methanation of CO and CO₂

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微地震监测技术探究

唐春华,顾广庆

《中国工程科学》 2012年第14卷第4期页码 95-99

摘要：

微地震监测是地球物理学中的一个重要研究方向，它在油田勘探开采等众多领域有广泛的应用。从微地震的形成机理出发，介绍了微地震的发展历程。重点讨论了微地震监测系统的重要组成部分、关键技术和微地震监测的具体实施，最后讨论了微地震未来的发展与趋势。

关键词：微地震监测水力压裂石油天然气信噪比事件定位

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以净零排放为目标的封存驱动型CO2sub>提高采收率方法 Article

刘月亮, 芮振华

《工程（英文）》 2022年第18卷第11期页码 79-87 doi: 10.1016/j.eng.2022.02.010

摘要：可通过驱油过程将CO2sub>封存在油藏地质体中，因此，CO2sub>驱油与封存被视为降低CO2sub>排放的重要手段之一。2sub>净零排放甚至负排放，同时最大限度提高原油采收率。该方法以二甲醚（DME）作为一种高效化学助剂，用于辅助传统CO2sub> 驱提高原油采收率，同时提高CO2sub>封存率。封存驱动型CO2sub> EOR方法在提高波及效率方面优于传统的CO2sub> EOR，尤其是在采油后期更为明显；同时，封存驱动型CO2sub> EOR比传统的通过优化开发方案，如水气交替注入，可实现更高的原油采收率和CO2sub>封存率目标。

关键词： CO2sub> EOR CO2sub>净排放量二甲醚封存驱动型CO2sub> EOR CO2sub>封存

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非均质储层CO2sub>泡沫调驱注入参数优化实验研究

赵金省,谭俊领,古正富,刘笑春

《中国工程科学》 2012年第14卷第11期页码 88-93

摘要：在此基础上，采用渗透率级差接近的两组并联岩心，进行了注入方式和注入段塞组合的优化实验。结果表明，地下起泡方式，即CO2和起泡剂交替注入的方式可以在高渗透层中形成较高的封堵压差，具有较好的驱油效果。最优的段塞组合是0.2倍孔隙体积的起泡剂+0.4倍孔隙体积的CO2气体，总注入段塞是0.6倍孔隙体积。

关键词：非均质储层 CO2sub>泡沫调驱注入参数实验研究

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页岩储层网络压裂技术研究与试验

贾长贵,,李双明,王海涛,蒋廷学

《中国工程科学》 2012年第14卷第6期页码 106-112

摘要：

页岩储层压裂技术是页岩油气高效勘探开发的关键技术和核心技术。与常规低渗油气储层压裂单一长缝改善压裂效果不同，低孔极低渗的页岩压裂主要目标是形成具有有效导流能力的网络裂缝，确保压裂改造体积足够大，且经济有效。提出了页岩网络压裂有效改造体积（ESRV）的概念。在借鉴北美页岩气压裂的经验和前期国内页岩气压裂实践的基础上，针对我国页岩储层的具体特点，在压前进行评价方法、射孔参数优化、诱导复合测试压裂、网络压裂对策和排采技术等方面进行了探索性的研究，初步形成了页岩网络压裂技术，现场试验效果明显，解决了裂缝性脆性页岩压裂易砂堵、成功率低的难题。

关键词：页岩储层网络压裂

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Frontier science and challenges on offshore carbon storage

《环境科学与工程前沿（英文）》 2023年第17卷第7期 doi: 10.1007/s11783-023-1680-6

摘要：

● The main direct seal up carbon options and challenges are reviewed.

关键词： Offshore carbon storage Direct CO₂ injection CO₂-CH₄ replacement CO₂-EOR CCS hubs CO₂ transport

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Reduction potential of the energy penalty for CO capture in CCS

《能源前沿（英文）》 2023年第17卷第3期页码 390-399 doi: 10.1007/s11708-023-0864-x

摘要： CO₂ capture and storage (CCS) has been acknowledged as an essential part of a portfolio of technologies that are required to achieve cost-effective long-term CO₂ mitigation. However, the development progress of CCS technologies is far behind the targets set by roadmaps, and engineering practices do not lead to commercial deployment. One of the crucial reasons for this delay lies in the unaffordable penalty caused by CO₂ capture, even though the technology has been commonly recognized as achievable. From the aspects of separation and capture technology innovation, the potential and promising direction for solving this problem were analyzed, and correspondingly, the possible path for deployment of CCS in China was discussed. Under the carbon neutral target recently proposed by the Chinese government, the role of CCS and the key milestones for deployment were indicated.

关键词： CO₂ capture and storage (CCS) CO₂ separation energy penalty

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Al2sub>O3sub> and CeO2sub>-promoted MgO sorbents for CO2sub> capture at moderate

Huimei Yu, Xiaoxing Wang, Zhu Shu, Mamoru Fujii, Chunshan Song

《化学科学与工程前沿（英文）》 2018年第12卷第1期页码 83-93 doi: 10.1007/s11705-017-1691-6

摘要： A series of Al O and CeO modified MgO sorbents was prepared and studied for CO sorption at moderate temperatures. The CO sorption capacity of MgO was enhanced with the addition of either Al O or CeO . Over Al O -MgO sorbents, the best capacity of 24.6 mg-CO /g-sorbent was attained at 100 °C, which was 61% higher than that of MgO (15.3 mg-CO /g-sorbent). The highest capacity of 35.3 mg-CO /g-sorbent was obtained over the CeO -MgO sorbents at the optimal temperature of 200 °C. Combining with the characterization results, we conclude that the promotion effect on CO sorption with the addition of Al O and CeO can be attributed to the increased surface area with reduced MgO crystallite size. Moreover, the addition of CeO increased the basicity of MgO phase, resulting in more increase in the CO capacity than Al O promoter. Both the Al O -MgO and CeO -MgO sorbents exhibited better cyclic stability than MgO over the course of fifteen CO sorption-desorption cycles. Compared to Al O , CeO is more effective for promoting the CO capacity of MgO. To enhance the CO capacity of MgO sorbent, increasing the basicity is more effective than the increase in the surface area.

关键词： CO₂ capture MgO sorbents Al₂O₃ CeO₂ flue gas

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ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

《化学科学与工程前沿（英文）》 2017年第11卷第2期页码 197-204 doi: 10.1007/s11705-016-1606-y

摘要： ZnFe O -BiOCl composites were prepared by both hydrothermal and direct precipitation processes and the structures and properties of the samples were characterized by various instrumental techniques. The samples were then used as catalysts for the photocatalytic reduction of CO in cyclohexanol under ultraviolet irradiation to give cyclohexanone (CH) and cyclohexyl formate (CF). The photocatalytic CO reduction activities over the hydrothermally prepared ZnFe O -BiOCl composites were higher than those over the directly-precipitated composites. This is because compared to the direct-precipitation sample, the ZnFe O nanoparticles in the hydrothermal sample were smaller and more uniformly distributed on the surface of BiOCl and so more heterojunctions were formed. Higher CF and CH yields were obtained for the pure BiOCl and BiOCl composite samples with more exposed (001) facets than for the samples with more exposed (010) facets. This is due to the higher density of oxygen atoms in the exposed (001) facets, which creates more oxygen vacancies, and thereby improves the separation efficiency of the electron-hole pairs. More importantly, irradiation of the (001) facets with ultraviolet light produces photo-generated electrons which is helpful for the reduction of CO to ·CO . The mechanism for the photocatalytic reduction of CO in cyclohexanol over ZnFe O -BiOCl composites with exposed (001) facets involves electron transfer and carbon radical formation.

关键词： reduction of CO₂ cyclohexanol ZnFe₂O₄ deposited BiOCl facet composite photocatalyst